The alleged incident happened on the carousel at the Dreamland Amusements carnival at the Smith Haven Mall in Lake Grove around 7 p.m. Wednesday.
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Authorities say the 7-year-old victim was riding the merry-go-round when the operator, 50-year-old Louis Shelton, of King of Prussia, Pennsylvania, inappropriately touched her.
Suffolk County police Detective Sergeant Joseph Isnardi said Shelton was securing the girl on the carousel when the incident happened, but that the mechanism he used to strap her in did not warrant his hands being near her genitalia.
"There was no valid excuse for the hand to have gone where it went," Isnardi said.
Two other people on the ride witnessed the incident and called police.
Officers responded and placed Shelton under arrest.
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Police interviewed the two witnesses and the girl, who was there with her parents.
Shelton is charged with first-degree sexual abuse and endangering the welfare of child.
He is being held on $15,000 bail and is due back in court on June 11.
Detectives are asking anyone with information or who believes they may be a victim to call the Special Victim's Section at 631-852-6184.